It sounds like you just want to rev it high. The point being is you don’t need RPM to achieve a good ET if that is your goal. You can make 350-360RWHP at a safer RPM with more mid range torque on top vs moving the peak up a few hundred RPM. Also, dyno runs from 3k up at WOT aren’t showing the significant low end losses you would see during street driving with more aggressive cams. This also happens with NSR cams, just not as pronounced.
If you want to rev it above 7K reliably, you will want a stronger rod than the factory powdered rods. At those engine speeds, the stress on the rods increases exponentially.
There isn't a single aftermarket cam that'll outperform the stock cam from idle to 4400rpm, and all will sacrifice torque below that rpm to some degree. If you also add an aftermarket intake manifold, the combination of cams/manifold essentially takes a hit to the torque curve below 5000rpm and adds torque above that. This is Four Eyes before and after adding Detroit Rocker cams and the Ford Performance IM.
The stock powdered metal rods are light and strong enough for 7000rpm in a N/A 4.6 but for insurance and peace of mind, I'd prefer the Gen 2/3 Coyote (same as Boss 302) rods if anything nearer 7500rpm is the goal. You'd also need to consider a higher capacity oil pan and HV pump with billet gears for 7500rpm. Sustained engine speeds of 6500rpm & above will require locked out phasers to prevent their failure.
If you're looking for ~360rwhp your peak HP is going to be at or near 6500rpm with peak torque of ~330rwtq arriving at or near 5000rpm. The dyno graphs I posted tell the story. Therefore you'll want to rev the engine up to 7000 if you're going to exploit the extra top end performance. If you want a strong 2500-4500rpm midrange for street use, stick with the stock cams & IM with delete plates and settle for a ~6500rpm limit.
Dollars to doughnuts the Livernois stage 2 cams your looking at are in fact the Comp cams 127500s in a Livernois box. That being the case you will have to lock the phasers and run the springs recommended by the manufacture. Don’t forget the retainers. If Livernois springs meet the manufactures spec. they should work. I still think 4.10s would be a good choice for the rear. I would match that cam with as much compression as I could get away with. 11 to 1 with good fuel and a Lito tune.
With a stock 3.542" stroke you'll have a hard time finding a piston that'll give you much above 10.0:1 compression, and 11.0:1 is only possible with a longer stroke i.e. stroker build. With the high valve lift of SPR cams, you'd need to verify PTV clearance and lock out the phasers altogether if you zero deck the block and use flat top pistons for a higher compression ratio. This is where going down the rabbit hole of a maximum effort N/A build with CNC ported stage 3 heads (1mm oversize valves) gets really expensive to the point where it only makes sense if you have a YouTube channel with over 100k subscribers to fund the project! By this stage you're going to need 4.10 or even 4.30 ratio axle gears to make the sacrifice of lower rpm torque somewhat acceptable.
At the end of the day the 3V is a very good engine but it can never match the performance of a Coyote across a wider 1500-7500rpm range even when built as an 10.2:1 compression 301ci stroker (Four Eyes again

) simply because it's constrained by a single exhaust valve per cylinder, a single camshaft on each bank and, consequently, the inability to vary the lobe separation angle as well as the intake/exhaust centerline angles in order to widen the power band. Once you lock the cam phasers, the power band becomes even narrower.
Therefore it's important to recognise those constraints and try to make the best of what you have without sacrificing too much drivability for the sake of having a 7000+rpm screamer.